Imaging the homogeneous nucleation during the melting of superheated colloidal crystals | |
Wang ZR; Wang F; Peng Y; Zheng ZY(郑中玉); Han YL; Han, YL; Hong Kong Univ Sci & Technol, Dept Phys, Hong Kong, Hong Kong, Peoples R China. | |
发表期刊 | SCIENCE |
2012-10-05 | |
卷号 | 338期号:6103页码:87-90 |
ISSN | 0036-8075 |
摘要 | The nucleation process is crucial to many phase transitions, but its kinetics are difficult to predict and measure. We superheated and melted the interior of thermal-sensitive colloidal crystals and investigated by means of video microscopy the homogeneous melting at single-particle resolution. The observed nucleation precursor was local particle-exchange loops surrounded by particles with large displacement amplitudes rather than any defects. The critical size, incubation time, and shape and size evolutions of the nucleus were measured. They deviate from the classical nucleation theory under strong superheating, mainly because of the coalescence of nuclei. The superheat limit agrees with the measured Born and Lindemann instabilities. |
关键词 | Phase-transition Stability Limit Catastrophe Science Growth Bulk |
学科领域 | 流体力学 |
URL | 查看原文 |
收录类别 | SCI |
语种 | 英语 |
WOS记录号 | WOS:000309457400058 |
项目资助者 | This work was supported by the Research Grants Council of Hong Kong (General Research Fund 601208 and 601911), and we thank A. Alsayed and A. Yodh for providing the NIPA colloids. |
课题组名称 | NML空间材料物理力学 |
论文分区 | 一类 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://dspace.imech.ac.cn/handle/311007/46586 |
专题 | 微重力重点实验室 |
通讯作者 | Han, YL; Hong Kong Univ Sci & Technol, Dept Phys, Hong Kong, Hong Kong, Peoples R China. |
推荐引用方式 GB/T 7714 | Wang ZR,Wang F,Peng Y,et al. Imaging the homogeneous nucleation during the melting of superheated colloidal crystals[J]. SCIENCE,2012,338,6103,:87-90. |
APA | Wang ZR.,Wang F.,Peng Y.,Zheng ZY.,Han YL.,...&Hong Kong Univ Sci & Technol, Dept Phys, Hong Kong, Hong Kong, Peoples R China..(2012).Imaging the homogeneous nucleation during the melting of superheated colloidal crystals.SCIENCE,338(6103),87-90. |
MLA | Wang ZR,et al."Imaging the homogeneous nucleation during the melting of superheated colloidal crystals".SCIENCE 338.6103(2012):87-90. |
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