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Synthesis and hydrogen-storage performance of interpenetrated MOF-5/MWCNTs hybrid composite with high mesoporosity
Jiang H(姜恒); Feng YF(冯亚菲); Chen M(陈猛); Wang YR(王育人); Wang, YR (reprint author), Chinese Acad Sci, Inst Mech, Key Lab Micrograv Sci, Beijing 100190, Peoples R China.
Source PublicationInternational Journal of Hydrogen Energy
2013-08-21
Volume38Issue:25Pages:10950-10955
ISSN0360-3199
AbstractMetal-organic frameworks (MOFs) exhibiting high surface area and tunable pore size own broad application prospects. Compared with existing MOFs, MOF-5 [Zn4O(bdc)3] is a promising hydrogen storage material due to high H2 uptake capacity and thermostability. However, further wider applications of MOF-5 have been limited because atmospheric moisture levels cause MOF-5 instability. MOF-5 and multi-walled carbon nanotubes (MWCNTs) hybrid composite (denoted MOFMC) can enhance stability toward ambient moisture and improve hydrogen storage capacity. In this paper, the MOFMC, which has an interpenetrated structure with high mesoporosity, was synthesized. The MOFMC is denoted as Int-MOFMC-meso. It stored 2.02 wt% H2 at 77 K under 1 bar, which is higher than the MOF-5 with similar structure and the earlier reported MOFMC material. Moreover, the Int-MOFMC-meso can also show more excellent performance of thermostability and moisture stability than the MOF-5 with similar structure.
KeywordMetal-organic Frameworks Interpenetrated Structure Hydrogen-storage Multi-walled Carbon Nanotubes High Mesoporosity
Subject Area新型材料的力学问题
DOI10.1016/j.ijhydene.2013.03.044
URL查看原文
Indexed BySCI ; EI
Language英语
WOS IDWOS:000324563100096
WOS KeywordMETAL-ORGANIC FRAMEWORKS ; NANOPOROUS MATERIALS ; SORPTION PROPERTIES ; ADSORPTION ; CARBON ; MOF-5 ; INCLUSION ; BEHAVIORS ; DESIGN ; SIZE
WOS Research AreaChemistry ; Electrochemistry ; Energy & Fuels
WOS SubjectChemistry, Physical ; Electrochemistry ; Energy & Fuels
Funding OrganizationThe authors wish to acknowledge the support from the National Natural Science Foundation of China (Nos. 11202211 and 11272315).
Department中科院国家微重力实验室
Citation statistics
Cited Times:27[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://dspace.imech.ac.cn/handle/311007/47434
Collection国家微重力实验室
Corresponding AuthorWang, YR (reprint author), Chinese Acad Sci, Inst Mech, Key Lab Micrograv Sci, Beijing 100190, Peoples R China.
Recommended Citation
GB/T 7714
Jiang H,Feng YF,Chen M,et al. Synthesis and hydrogen-storage performance of interpenetrated MOF-5/MWCNTs hybrid composite with high mesoporosity[J]. International Journal of Hydrogen Energy,2013,38(25):10950-10955.
APA 姜恒,冯亚菲,陈猛,王育人,&Wang, YR .(2013).Synthesis and hydrogen-storage performance of interpenetrated MOF-5/MWCNTs hybrid composite with high mesoporosity.International Journal of Hydrogen Energy,38(25),10950-10955.
MLA 姜恒,et al."Synthesis and hydrogen-storage performance of interpenetrated MOF-5/MWCNTs hybrid composite with high mesoporosity".International Journal of Hydrogen Energy 38.25(2013):10950-10955.
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