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Fluorescent components and spatial patterns of chromophoric dissolved organic matters in Lake Taihu, a large shallow eutrophic lake in China
Yao B(姚波); Hu CM(胡春明); Liu QQ(刘青泉); Yao, B (reprint author), Chinese Acad Sci, Inst Mech, Key Lab Mech Fluid Solid Coupling Syst, Beijing 100190, Peoples R China.
发表期刊ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
2016
卷号23期号:22页码:23057-23070
ISSN0944-1344
摘要Water samples at both surface and bottom layers were taken from 102 sites in Lake Taihu to study the fluorescent components and spatial patterns of chromophoric dissolved organic matters (CDOM). Three-dimensional excitation-emission matrix data obtained from the samples were analyzed by parallel factor approach in which four humic-like and two protein-like fluorescent components (named C1-C6) were identified. The results showed that fluorescence intensities were higher in the northern and western lake regions, and notable declines of fluorescence maxima (F (max)) were observed from the northwest to the center and then to the southeast of the lake. Calculated biological index (BIX) values ranged from 0.88 to 1.44 and humification index (HIX) values from 0.64 to 3.37 for all the samples. The spatial variations of BIX and HIX values suggested stronger allochthonous CDOM characteristics in Zhushan Bay and the western area and autochthonous characteristics in the southern and eastern areas. Vertically, the average F (max) value of the surface samples was about 6 % less than that of the bottom samples, but noticeable variations existed among different sampling sites and components. These distribution characteristics of CDOM were mainly attributed to the spatial heterogeneity of sources and wind-induced transportation process. Interestingly, the C6 component (Ex(max)/Em(max) = 250/455 nm) seemed to be unique in samples from Zhushan Bay and probably resulted from the discharge of the Taige River. Therefore, it could be used as an indicator of point-source discharge and a tracer to study the fate of CDOM in the lake.
关键词Parafac Cdom Spatial Heterogeneity Vertical Difference Hydrodynamics
DOI10.1007/s11356-016-7510-7
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收录类别SCI ; EI
语种英语
WOS记录号WOS:000387602800074
关键词[WOS]PARAFAC ; CDOM ; Spatial heterogeneity ; Vertical difference ; Hydrodynamics
WOS研究方向Environmental Sciences & Ecology
WOS类目Environmental Sciences
项目资助者National Natural Science Foundation of China [11202217]
课题组名称LMFS水环境流体力学(LEM)
论文分区二类
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被引频次:12[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://dspace.imech.ac.cn/handle/311007/59954
专题流固耦合系统力学重点实验室
通讯作者Yao, B (reprint author), Chinese Acad Sci, Inst Mech, Key Lab Mech Fluid Solid Coupling Syst, Beijing 100190, Peoples R China.
推荐引用方式
GB/T 7714
Yao B,Hu CM,Liu QQ,et al. Fluorescent components and spatial patterns of chromophoric dissolved organic matters in Lake Taihu, a large shallow eutrophic lake in China[J]. ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,2016,23,22,:23057-23070.
APA 姚波,胡春明,刘青泉,&Yao, B .(2016).Fluorescent components and spatial patterns of chromophoric dissolved organic matters in Lake Taihu, a large shallow eutrophic lake in China.ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,23(22),23057-23070.
MLA 姚波,et al."Fluorescent components and spatial patterns of chromophoric dissolved organic matters in Lake Taihu, a large shallow eutrophic lake in China".ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH 23.22(2016):23057-23070.
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