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Mechanical Relaxation-to-Rejuvenation Transition in a Zr-based Bulk Metallic Glass
Zhang M(张猛); Wang YM; Li FX; Jiang SQ; Li MZ; Liu L; Liu, L (reprint author), Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, Wuhan 430074, Peoples R China.
发表期刊SCIENTIFIC REPORTS
2017-04-04
卷号7
ISSN2045-2322
摘要The relaxation of amorphous materials i.e. aging would largely endanger their performances in service. Here we report a mechanical relaxation-to-rejuvenation transition of a Zr35Ti30Be27.Cu-5(7.5) bulk metallic glass (BMG) in elastostatic compression at ambient temperature thus provide an accessible way to tailor the mechanical properties of amorphous materials. To unravel the structural evolution underlying the observed transition atomistic simulations parallel with the experimental tests on a typical model glass system Zr60Cu40 were performed which successfully reproduced and thus upheld the experimentally observed mechanical relaxation-to-rejuvenation transition. The variations of coordination number and atomic volume during the transition are evaluated to indicate a de-mixing tendency of the constituent atoms in the rejuvenation stage. This de-mixing tendency largely explains the difference between mechanical rejuvenation and thermal rejuvenation and reveals a competitive relationship between activation enthalpy and activation entropy in the stress-driven temperatureassisted atomic dynamics of BMG such as diffusion and plastic deformation etc.
DOI10.1038/s41598-017-00768-7
收录类别SCI
语种英语
WOS记录号WOS:000398162600001
关键词[WOS]AMORPHOUS-ALLOYS ; ELASTOSTATIC COMPRESSION ; STRUCTURAL RELAXATION ; SUPERCOOLED LIQUIDS ; TEMPERATURE ; FLOW ; DEFORMATION ; DYNAMICS ; BEHAVIOR
WOS研究方向Science & Technology - Other Topics
WOS类目Multidisciplinary Sciences
项目资助者National Nature Science Foundation of China(51531003 ; MOST 973 Program(2015CB856801) ; 51471074)
课题组名称LNM冲击动力学与新型材料力学性能
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力学所作者排名1
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被引频次:48[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://dspace.imech.ac.cn/handle/311007/60560
专题非线性力学国家重点实验室
通讯作者Liu, L (reprint author), Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, Wuhan 430074, Peoples R China.
推荐引用方式
GB/T 7714
Zhang M,Wang YM,Li FX,et al. Mechanical Relaxation-to-Rejuvenation Transition in a Zr-based Bulk Metallic Glass[J]. SCIENTIFIC REPORTS,2017,7.
APA 张猛.,Wang YM.,Li FX.,Jiang SQ.,Li MZ.,...&Liu, L .(2017).Mechanical Relaxation-to-Rejuvenation Transition in a Zr-based Bulk Metallic Glass.SCIENTIFIC REPORTS,7.
MLA 张猛,et al."Mechanical Relaxation-to-Rejuvenation Transition in a Zr-based Bulk Metallic Glass".SCIENTIFIC REPORTS 7(2017).
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