Modeling diffusion-induced stress on two-phase lithiation in lithium-ion batteries | |
Wu H1; Xie ZC2; Wang Y3,4; Lu CS4; Ma ZS1 | |
发表期刊 | EUROPEAN JOURNAL OF MECHANICS A-SOLIDS |
2018-09-01 | |
卷号 | 71页码:320-325 |
ISSN | 0997-7538 |
摘要 | Capacity fade induced by chemo-mechanical degradation during charge-discharge cycles is the bottleneck in the design of high-performance batteries, especially high-capacity electrode materials. In this paper, a flexible sigmoid function is used to create the two-phase electrochemical lithiation profile, describing a sharp phase boundary that separates the pristine core from the lithiated shell of an electrode particle. According to such a phase transition, an analytical solution of the stress evolution is obtained by introducing an electrochemical reaction layer into the plastic model. Finally, based on the theory of diffusion-induced stress and the energy principle, we determine the critical thickness of radius of a lithiated layer, at which fracture occurs. |
关键词 | Lithium-ion Battery Two-phase Lithiation Fracture Critical Size |
DOI | 10.1016/j.euromechsol.2018.04.005 |
收录类别 | SCI ; EI |
语种 | 英语 |
WOS记录号 | WOS:000440116300024 |
关键词[WOS] | Long Cycle Life ; Silicon Electrodes ; Crystalline Silicon ; Electrochemical Lithiation ; Initial Lithiation ; Amorphous-silicon ; Hollow Cylinder ; Thin-films ; Deformation ; Nanowires |
WOS研究方向 | Mechanics |
WOS类目 | Mechanics |
项目资助者 | National Natural Science Foundation of China(11372267 ; 11402086 ; 11472141) |
论文分区 | 一类 |
力学所作者排名 | 2 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://dspace.imech.ac.cn/handle/311007/77647 |
专题 | 非线性力学国家重点实验室 |
通讯作者 | Ma ZS |
作者单位 | 1.Xiangtan Univ, Natl Prov Lab Special Funct Thin Film Mat, Sch Mat Sci & Engn, Xiangtan 411105, Hunan, Peoples R China 2.Chinese Acad Sci, Inst Mech, State Key Lab Nonlinear Mech, Beijing 100190, Peoples R China 3.Hunan Univ Sci & Technol, Sch Informat & Elect Engn, Xiangtan 411201, Hunan, Peoples R China 4.Curtin Univ, Dept Mech Engn, Perth, WA 6845, Australia |
推荐引用方式 GB/T 7714 | Wu H,Xie ZC,Wang Y,et al. Modeling diffusion-induced stress on two-phase lithiation in lithium-ion batteries[J]. EUROPEAN JOURNAL OF MECHANICS A-SOLIDS,2018,71:320-325. |
APA | Wu H,Xie ZC,Wang Y,Lu CS,&Ma ZS.(2018).Modeling diffusion-induced stress on two-phase lithiation in lithium-ion batteries.EUROPEAN JOURNAL OF MECHANICS A-SOLIDS,71,320-325. |
MLA | Wu H,et al."Modeling diffusion-induced stress on two-phase lithiation in lithium-ion batteries".EUROPEAN JOURNAL OF MECHANICS A-SOLIDS 71(2018):320-325. |
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