Modeling NO and SO2 Oxidation by H2O2 in Coal-Fired Flue Gas

doi:10.1061/(ASCE)EE.1943-7870.0001458

	Modeling NO and SO2 Oxidation by H2O2 in Coal-Fired Flue Gas
	Li S(李森); Ge YF(葛逸飞); Wei XL(魏小林)
发表期刊	JOURNAL OF ENVIRONMENTAL ENGINEERING
	2018-11-01
卷号	144 期号:11 页码:4018113
ISSN	0733-9372
摘要	NO and SO2 oxidization by H2O2 in coal-fired flue gas was modeled, and the effects of temperature and H2O2 concentration on NO and SO2 oxidization were investigated. The pathways of NO and SO2 oxidization were as follows: H2O2OHHO2+NONO2 and SO2+OHHOSO2+O2SO3, respectively. There were optimal temperature ranges of NO and SO2 oxidization, and the ranges were 650-920K and 650-750K, respectively. In the optimal temperature ranges, the NO2 conversion rate was greater than 0.9 at MRH2O2/NO>1.9, and the SO3 conversion rate reached about 0.3 at MRH2O2/SO2=0.1-0.4. SO2 oxidization could promote HO2 formation to oxidize NO.
关键词	Hydrogen peroxide Oxidization Nitric oxide NO2 SO2
DOI	10.1061/(ASCE)EE.1943-7870.0001458
URL	查看原文
收录类别	SCI ; EI
语种	英语
WOS记录号	WOS:000444530900004
关键词[WOS]	HYDROGEN-PEROXIDE ; PHASE OXIDATION ; NITRIC-OXIDE ; EMISSIONS
WOS研究方向	Engineering, Environmental ; Engineering, Civil ; Environmental Sciences
WOS类目	Engineering ; Environmental Sciences & Ecology
项目资助者	National Natural Science Foundation of China [51376189] ; National Key Research and Development Plan of China [2016YFB0601503]
论文分区	Q3
力学所作者排名	1
引用统计	被引频次：9[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://dspace.imech.ac.cn/handle/311007/77928
专题	高温气体动力学国家重点实验室
作者单位	1.Chinese Acad Sci, Inst Mech, State Key Lab High Temp Gas Dynam, 15 Beisihuanxi Rd, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Sch Engn Sci, Beijing 100190, Peoples R China
推荐引用方式 GB/T 7714	Li S,Ge YF,Wei XL. Modeling NO and SO2 Oxidation by H2O2 in Coal-Fired Flue Gas[J]. JOURNAL OF ENVIRONMENTAL ENGINEERING,2018,144,11,:4018113.
APA	李森,葛逸飞,&魏小林.(2018).Modeling NO and SO2 Oxidation by H2O2 in Coal-Fired Flue Gas.JOURNAL OF ENVIRONMENTAL ENGINEERING,144(11),4018113.
MLA	李森,et al."Modeling NO and SO2 Oxidation by H2O2 in Coal-Fired Flue Gas".JOURNAL OF ENVIRONMENTAL ENGINEERING 144.11(2018):4018113.

条目包含的文件		下载所有文件
文件名称/大小	文献类型	版本类型	开放类型	使用许可
IrJ2018316.pdf（977KB）	期刊论文	出版稿	开放获取	CC BY-NC-SA	浏览下载