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Modeling NO and SO2 Oxidation by H2O2 in Coal-Fired Flue Gas
Li S(李森); Ge YF(葛逸飞); Wei XL(魏小林)
2018-11-01
发表期刊JOURNAL OF ENVIRONMENTAL ENGINEERING
卷号144期号:11页码:4018113
ISSN0733-9372
摘要NO and SO2 oxidization by H2O2 in coal-fired flue gas was modeled, and the effects of temperature and H2O2 concentration on NO and SO2 oxidization were investigated. The pathways of NO and SO2 oxidization were as follows: H2O2OHHO2+NONO2 and SO2+OHHOSO2+O2SO3, respectively. There were optimal temperature ranges of NO and SO2 oxidization, and the ranges were 650-920K and 650-750K, respectively. In the optimal temperature ranges, the NO2 conversion rate was greater than 0.9 at MRH2O2/NO>1.9, and the SO3 conversion rate reached about 0.3 at MRH2O2/SO2=0.1-0.4. SO2 oxidization could promote HO2 formation to oxidize NO.
关键词Hydrogen peroxide Oxidization Nitric oxide NO2 SO2
DOI10.1061/(ASCE)EE.1943-7870.0001458
URL查看原文
收录类别SCI ; EI
语种英语
WOS记录号WOS:000444530900004
关键词[WOS]HYDROGEN-PEROXIDE ; PHASE OXIDATION ; NITRIC-OXIDE ; EMISSIONS
WOS研究方向Engineering, Environmental ; Engineering, Civil ; Environmental Sciences
WOS类目Engineering ; Environmental Sciences & Ecology
项目资助者National Natural Science Foundation of China [51376189] ; National Key Research and Development Plan of China [2016YFB0601503]
论文分区Q3
力学所作者排名1
引用统计
文献类型期刊论文
条目标识符http://dspace.imech.ac.cn/handle/311007/77928
专题高温气体动力学国家重点实验室
作者单位1.Chinese Acad Sci, Inst Mech, State Key Lab High Temp Gas Dynam, 15 Beisihuanxi Rd, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, Sch Engn Sci, Beijing 100190, Peoples R China
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GB/T 7714
Li S,Ge YF,Wei XL. Modeling NO and SO2 Oxidation by H2O2 in Coal-Fired Flue Gas[J]. JOURNAL OF ENVIRONMENTAL ENGINEERING,2018,144(11):4018113.
APA 李森,葛逸飞,&魏小林.(2018).Modeling NO and SO2 Oxidation by H2O2 in Coal-Fired Flue Gas.JOURNAL OF ENVIRONMENTAL ENGINEERING,144(11),4018113.
MLA 李森,et al."Modeling NO and SO2 Oxidation by H2O2 in Coal-Fired Flue Gas".JOURNAL OF ENVIRONMENTAL ENGINEERING 144.11(2018):4018113.
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