IMECH-IR  > 国家微重力实验室
A Research on Preparation and Application of the Monolithic Catalyst with Interconnecting Pore Structure
Tsai SB; Ma HL
发表期刊SCIENTIFIC REPORTS
2018-11-09
卷号8页码:Ar-16605
ISSN2045-2322
摘要In recent years, the monolithic material has been developed increasingly in the high performance liquid phase field, and it could also be applied in the field of catalyst, as a monolithic catalyst carrier, since it has a large specific surface area, and could be customized based on the mould. The monolithic catalyst is characterized with many advantages such as low bed pressure, high physical efficiency and small amplification effect. The most impotant part refers to the preparation of copper-based catalyst. The impregnation method is used to produce CuO-ZnO monolithic catalyst and CuO-ZnO-ZrO2 monolithic catalyst with the prepared monolithic silica-alumina carrier. The fixed bed microreactor is used to investigate the effect of copper-based catalyst on the process in which carbon dioxide is used to produce methanol through hydrogenation. The metal salt is added into the sol-gel process, which could form the M-O-Si bond, thus make the metal-containing catalytic material obtain good mechanical strength, and make it possible to be introduced into the acidic center generally. The metal-containing catalytic material carrier also has macropores and mesopores. The presence of large pores could make the molecular mass transfer more effective, while the presence of mesopores could increase the specific surface area of the material. In this paper, the experimental study has been conducted on the production of methanol through hydrogenation of CO2 under different catalysts, to mainly investigate the effect of catalysts with different catalytic performance on the reaction.
DOI10.1038/s41598-018-35021-2
URL查看原文
收录类别SCI
语种英语
WOS记录号WOS:000449632300014
关键词[WOS]SOL-GEL PROCESS ; PHASE-SEPARATION ; SILICA ; MACROPORES
WOS研究方向Multidisciplinary Sciences
WOS类目Science & Technology - Other Topics
项目资助者2018 Zhongshan Innovation and Development Research Center
论文分区二类/Q1
力学所作者排名2
引用统计
文献类型期刊论文
条目标识符http://dspace.imech.ac.cn/handle/311007/78163
专题国家微重力实验室
作者单位1.Univ Elect Sci & Technol China, Zhongshan Inst, Zhongshan 528402, Guangdong, Peoples R China
2.Civil Aviat Univ China, Res Ctr Environm & Sustainable Dev China Civil Av, Tianjin 300300, Peoples R China
3.Chinese Acad Sci, Inst Mech, Beijing 100190, Peoples R China
4.Jinggangshan Univ, Sch Sci, Jian 343009, Jiangxi, Peoples R China
推荐引用方式
GB/T 7714
Tsai SB,Ma HL. A Research on Preparation and Application of the Monolithic Catalyst with Interconnecting Pore Structure[J]. SCIENTIFIC REPORTS,2018,8:Ar-16605.
APA Tsai SB,&Ma HL.(2018).A Research on Preparation and Application of the Monolithic Catalyst with Interconnecting Pore Structure.SCIENTIFIC REPORTS,8,Ar-16605.
MLA Tsai SB,et al."A Research on Preparation and Application of the Monolithic Catalyst with Interconnecting Pore Structure".SCIENTIFIC REPORTS 8(2018):Ar-16605.
条目包含的文件
条目无相关文件。
个性服务
推荐该条目
保存到收藏夹
查看访问统计
导出为Endnote文件
谷歌学术
谷歌学术中相似的文章
[Tsai SB]的文章
[Ma HL]的文章
百度学术
百度学术中相似的文章
[Tsai SB]的文章
[Ma HL]的文章
必应学术
必应学术中相似的文章
[Tsai SB]的文章
[Ma HL]的文章
相关权益政策
暂无数据
收藏/分享
所有评论 (0)
暂无评论
 

除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。