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Effects of water vapor and temperature on NOx and CO emissions during converter gas combustion
Zhai YH(翟英华); Li S(李森); Yan, WP; Wei XL(魏小林); Zhang, LY; Wang, YT
发表期刊FUEL
2019-11-15
卷号256页码:6
ISSN0016-2361
摘要

Converter gas is a valuable fuel in the converter steelmaking process, and NOx and CO emissions are high due to the high temperature combustion and the absence of H2O vapor. The effects of H2O vapor concentration and the inlet temperature of converter gas on NOx and CO emissions in the combustion are investigated by a detailed chemical reaction mechanism. CO emission decreases sharply when C-H2O,C-inlet increases from 0 to 0.4%. At C-H2O,C-inlet > 0.4% and T-inlet < 950 K, for the reduction of CO emission, the inlet temperature of converter gas is predominant over that of H2O vapor in air. The inlet temperature of converter gas has noticeable influence on NO emission at C-H2O,C-inlet < 2%. With the increase of C-H2O,C-inlet, NO emission first increases, then reaches a peak value, finally decreases. At T-inlet > 1050 K and C-H2O,C-inlet > 2%, NO emission noticeably decreases with C-H2O,C-inlet. In the presence of H2O, H and OH free radicals are easily formed, the reduction path of NO is as follows: NO -> NH/HNO -> N-2.

关键词Water vapor concentration Converter gas Inlet temperature CO emission NO emission
DOI10.1016/j.fuel.2019.115914
收录类别SCI ; EI
语种英语
WOS记录号WOS:000482184800039
关键词[WOS]NUMERICAL-SIMULATION ; METHANE
WOS研究方向Energy & Fuels ; Engineering
WOS类目Energy & Fuels ; Engineering, Chemical
资助项目Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences[XDA21040500]
项目资助者Transformational Technologies for Clean Energy and Demonstration, Strategic Priority Research Program of the Chinese Academy of Sciences
论文分区一类
力学所作者排名1
RpAuthorLi, Sen
引用统计
被引频次:9[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://dspace.imech.ac.cn/handle/311007/79964
专题高温气体动力学国家重点实验室
推荐引用方式
GB/T 7714
Zhai YH,Li S,Yan, WP,et al. Effects of water vapor and temperature on NOx and CO emissions during converter gas combustion[J]. FUEL,2019,256:6.
APA Zhai YH,Li S,Yan, WP,Wei XL,Zhang, LY,&Wang, YT.(2019).Effects of water vapor and temperature on NOx and CO emissions during converter gas combustion.FUEL,256,6.
MLA Zhai YH,et al."Effects of water vapor and temperature on NOx and CO emissions during converter gas combustion".FUEL 256(2019):6.
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