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Compact Assembly and Programmable Integration of Supercapacitors
Lu B1; Liu F(刘峰)2; Sun GQ1; Gao J1; Xu T1; Xiao YK1; Shao CX1; Jin XT1; Yang HS1; Zhao Y1; Zhang ZP1; Jiang L3; Qu LT1,4,5
发表期刊ADVANCED MATERIALS
2020-02
页码9
ISSN0935-9648
摘要

Microsized supercapacitors (mSCs) with small volume, rapid charge-discharge rate, and ultralong cyclic lifetime are urgently needed to meet the demand of miniaturized portable electronic devices. A versatile self-shrinkage assembling (SSA) strategy to directly construct the compact mSCs (CmSCs) from hydrogels of reduced graphene oxide is reported. A single CmSC is only 0.0023 cm(3) in volume, which is significantly smaller than most reported mSCs in fiber/yarn and planar interdigital forms. It exhibits a high capacitance of up to 68.3 F cm(-3) and a superior cycling stability with 98% capacitance retention after 25 & x202f;000 cycles. Most importantly, the SSA technique enables the CmSC as the building block to realize arbitrary, programmable, and multi-dimensional integration for adaptable and complicated power systems. By design on mortise and tenon joint connection, autologous integrated 3D interdigital CmSCs are fabricated in a self-holding-on manner, which thus dramatically reduces the whole device volume to achieve the high-performance capacitive behavior. Consequently, the SSA technique offers a universal and versatile approach for large-scale on-demand integration of mSCs as flexible and transformable power sources.

关键词high volumetric capacitance large-scale integration microsized supercapacitors mortise and tenon joints self-shrinkage assembly
DOI10.1002/adma.201907005
收录类别SCI ; EI
语种英语
WOS记录号WOS:000503090200001
关键词[WOS]ALL-SOLID-STATE ; MICRO-SUPERCAPACITORS ; GRAPHENE OXIDE ; ENERGY-STORAGE ; CARBON ; MICROSUPERCAPACITORS ; FABRICATION ; ELECTRODES ; ARRAYS
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
WOS类目Chemistry, Multidisciplinary ; Chemistry, Physical ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter
资助项目National Key R&D Program of China[2017YFB1104300] ; National Key R&D Program of China[2016YFA0200200] ; NSFC[11602272] ; NSFC[11972349] ; NSFC[51673026] ; NSFC[51433005] ; NSFC[21774015] ; NSFC[21604003] ; NSFC-STINT[21911530143] ; NSFC-MAECI[51861135202]
项目资助者National Key R&D Program of China ; NSFC ; NSFC-STINT ; NSFC-MAECI
论文分区一类
力学所作者排名2
RpAuthorQu, Liangti
引用统计
被引频次:45[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://dspace.imech.ac.cn/handle/311007/81289
专题非线性力学国家重点实验室
作者单位1.Beijing Inst Technol, Sch Chem & Chem Engn, Minist Educ China, Key Lab Cluster Sci,Key Lab Photoelect Electropho, Beijing 100081, Peoples R China;
2.Chinese Acad Sci, Inst Mech, State Key Lab Nonlinear Mech, Beijing 100190, Peoples R China;
3.Beijing Inst Technol, Sch Mech Engn, Laser Micro Nanofabricat Lab, Beijing 100081, Peoples R China;
4.Tsinghua Univ, Dept Mech Engn, State Key Lab Tribol, Key Lab Adv Mater Proc Technol,Minist Educ China, Beijing 100084, Peoples R China;
5.Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China
推荐引用方式
GB/T 7714
Lu B,Liu F,Sun GQ,et al. Compact Assembly and Programmable Integration of Supercapacitors[J]. ADVANCED MATERIALS,2020:9.
APA Lu B.,Liu F.,Sun GQ.,Gao J.,Xu T.,...&Qu LT.(2020).Compact Assembly and Programmable Integration of Supercapacitors.ADVANCED MATERIALS,9.
MLA Lu B,et al."Compact Assembly and Programmable Integration of Supercapacitors".ADVANCED MATERIALS (2020):9.
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