| Skeletal Nickel Catalyst for the Methanation Reaction Developed by Laser-Engineered Net-Shaping Technology | |
Yan, Kuo1; Lin, Zaiwen1; Li, Xu2; Chen M(陈猛)3,4 ; Wang, Xiaolong2; Wang YR(王育人)3,4; Wang, Jun1; Jiang H(姜恒)3,4
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| 通讯作者 | Lin, Zaiwen(linzaiwen@hrbeu.edu.cn) ; Jiang, Heng(hengjiang@imech.ac.cn) |
| 发表期刊 | CATALYSTS
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| 2022-02-01 | |
| 卷号 | 12期号:2页码:11 |
| 摘要 | Here, we report a skeletal nickel catalyst prepared by cumulative processing. The Ni, Al, and CoCrMo multi-component alloys were printed by a dual-powder laser-engineered net-shaping system, and alloy samples with different components were obtained through high-throughput design. After leaching in 5 mol/L NaOH at 40 degrees C for 2 h, the specific surface area of the catalyst increased with increasing Al content. Increasing the leaching temperature and prolonging the leaching time also effectively increased the specific surface area of the catalyst. After leaching at 80 degrees C for 12 h, the specific surface area was 42.36 m(2)/g. After cleaning and hydrogen-reduction treatment at 400 degrees C, the catalyst showed high catalytic activity. The highest conversion rate of CO reached 89.56%, and the selectivity of CH4 remained above 98% for a long time. |
| 关键词 | clean energy synthetic natural gas skeleton nickel 3D print |
| DOI | 10.3390/catal12020208 |
| 收录类别 | SCI |
| 语种 | 英语 |
| WOS记录号 | WOS:000771739100001 |
| 关键词[WOS] | CO METHANATION ; NI-CATALYST ; GAS |
| WOS研究方向 | Chemistry |
| WOS类目 | Chemistry, Physical |
| 资助项目 | National Natural Science Foundation of China[11972034] ; Beijing Research Program[Z171100000817010] ; Strategic Pilot Research Program of the Chinese Academy of Sciences[XDB22040301] |
| 项目资助者 | National Natural Science Foundation of China ; Beijing Research Program ; Strategic Pilot Research Program of the Chinese Academy of Sciences |
| 论文分区 | 二类 |
| 力学所作者排名 | 1 |
| RpAuthor | Lin, Zaiwen ; Jiang, Heng |
| 引用统计 | |
| 文献类型 | 期刊论文 |
| 条目标识符 | http://dspace.imech.ac.cn/handle/311007/88773 |
| 专题 | 微重力重点实验室 |
| 作者单位 | 1.Harbin Engn Univ, Coll Mat Sci & Chem Engn, Harbin 150001, Peoples R China; 2.Huaneng Clean Energy Res Inst, Beijing 102209, Peoples R China; 3.Chinese Acad Sci, Inst Mech, Key Lab Micrograv, Beijing 100190, Peoples R China; 4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yan, Kuo,Lin, Zaiwen,Li, Xu,et al. Skeletal Nickel Catalyst for the Methanation Reaction Developed by Laser-Engineered Net-Shaping Technology[J]. CATALYSTS,2022,12,2,:11. |
| APA | Yan, Kuo.,Lin, Zaiwen.,Li, Xu.,陈猛.,Wang, Xiaolong.,...&姜恒.(2022).Skeletal Nickel Catalyst for the Methanation Reaction Developed by Laser-Engineered Net-Shaping Technology.CATALYSTS,12(2),11. |
| MLA | Yan, Kuo,et al."Skeletal Nickel Catalyst for the Methanation Reaction Developed by Laser-Engineered Net-Shaping Technology".CATALYSTS 12.2(2022):11. |
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| 文件名称/大小 | 文献类型 | 版本类型 | 开放类型 | 使用许可 | ||
| Jp2022FA525_2022_Ske（6144KB） | 期刊论文 | 出版稿 | 开放获取 | CC BY-NC-SA | 浏览 下载 | |
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