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Viscoelastic Behavior and Constitutive Relation of Heavy Crude Oils
Liu, Hai-fei1,2; Xu, Yuan-yuan1; Chen, Hu3; Zhang J(张健)1,3; Xu JY(许晶禹)3
通讯作者Zhang, Jian(zhangjian@imech.ac.cn)
发表期刊ACS OMEGA
2022-08-25
页码7
ISSN2470-1343
摘要Heavy crude oil exhibits very complex viscoelastic behaviors due to its complex composition of resins, asphaltenes, saturates, and aromatics. It has a great influence on oil production and transportation. In this work, the viscoelastic behaviors of three different heavy crude oils were measured using a rotational rheometer. In conclusion, all of these heavy crude oils display linear viscoelastic behaviors in the experimental range. The loss modulus (E') of the three crude oils decreased as the experimental temperature increased, and the variation trends of the three crude oils were basically the same. However, the experimental temperature has almost no effect on the storage modulus (E'), which always retained a constant value of 0.4 Pa. Furthermore, the storage modulus (E') and loss modulus (E '') increase as the angular frequency increases. To describe the physical deformation characteristics of viscoelastic materials, the generalized Maxwell model and the fractional derivative Maxwell model are used to establish the constitutive relation of heavy crude oil. In conclusion, the generalized Maxwell model and the fractional derivative Maxwell model can predict the experimental results very well. All of the square of the correlation coefficient (R-2) values are greater than 0.95. However, the number of fitting parameters for the fractional derivative Maxwell model is less than that for the fourth-order generalized Maxwell model which can save the calculating time. Therefore, the fractional derivative Maxwell model is suggested to describe the viscoelastic behavior of heavy crude oil in industrial applications.
DOI10.1021/acsomega.2c02234
收录类别SCI
语种英语
WOS记录号WOS:000848467300001
关键词[WOS]RHEOLOGICAL BEHAVIOR ; MODELS ; TRANSITION ; SPECTRA ; FLOW
WOS研究方向Chemistry
WOS类目Chemistry, Multidisciplinary
资助项目State Key Laboratory of Technologies in Space Cryogenic Propellants[SKLTSCP202010] ; National Natural Science Foundation of China[11972039]
项目资助者State Key Laboratory of Technologies in Space Cryogenic Propellants ; National Natural Science Foundation of China
论文分区二类
力学所作者排名1
RpAuthorZhang, Jian
引用统计
文献类型期刊论文
条目标识符http://dspace.imech.ac.cn/handle/311007/90013
专题流固耦合系统力学重点实验室
作者单位1.State Key Lab Technol Space Cryogen Propellants, Beijing 100028, Peoples R China;
2.Beijing Inst Space Launch Technol, Beijing 100076, Peoples R China;
3.Chinese Acad Sci, Inst Mech, Beijing 100190, Peoples R China
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GB/T 7714
Liu, Hai-fei,Xu, Yuan-yuan,Chen, Hu,et al. Viscoelastic Behavior and Constitutive Relation of Heavy Crude Oils[J]. ACS OMEGA,2022:7.
APA Liu, Hai-fei,Xu, Yuan-yuan,Chen, Hu,张健,&许晶禹.(2022).Viscoelastic Behavior and Constitutive Relation of Heavy Crude Oils.ACS OMEGA,7.
MLA Liu, Hai-fei,et al."Viscoelastic Behavior and Constitutive Relation of Heavy Crude Oils".ACS OMEGA (2022):7.
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