Experimental investigation and numerical simulation of CO oxidation with HCl addition

doi:10.1016/j.fuel.2016.03.094

	Experimental investigation and numerical simulation of CO oxidation with HCl addition
	Wu, Dongyin; Wang, Yuhao; Wei XL(魏小林); Li S(李森); Guo, Xiaofeng; Wei, XL (reprint author), Chinese Acad Sci, Inst Mech, State Key Lab High Temp Gas Dynam, Beijing 100190, Peoples R China.
发表期刊	FUEL
	2016
卷号	179 页码:221-228
ISSN	0016-2361
摘要	Chlorine is rich in biomass and some coals and significantly released as HCl(g) during combustion process, and this promotes the recombination of free radicals OH, H, O, and HO2 and further influences CO oxidation. In this paper, the inhibition effect of HCl on CO oxidation is investigated by experiment and numerical simulation. The experiment is operated under different reaction zone temperatures and equivalence ratios in an entrained flow reactor. And the numerical simulation is conducted by CFD software coupled with reduced reaction mechanism. The results indicate that HCl addition obviously inhibits CO oxidation under oxygen-rich condition, and the inhibition enhances as HCl concentration rises, but weakens as temperature increases. Under chemical equivalent and oxygen-lean conditions, the inhibition effect is limited. (C) 2016 Elsevier Ltd. All rights reserved.
关键词	Inhibition Effect Co Oxidation Reduced Mechanism Hcl Efr
DOI	10.1016/j.fuel.2016.03.094
收录类别	SCI ; EI
语种	英语
WOS记录号	WOS:000374977300026
关键词[WOS]	FLUIDIZED-BED COMBUSTION ; TRACE QUANTITIES ; CHLORINE ; INHIBITION ; EMISSIONS ; NO ; COCOMBUSTION ; RELEASE ; BIOMASS ; STRAW
WOS研究方向	Energy & Fuels ; Engineering, Chemical
项目资助者	Financial support by National Natural Science Foundation of China (Project No. 91530112) is gratefully acknowledged. We also thank Dr. Jingwei Zhang for his test data and Prof. Glarborg in DTU for his help on reactor design.
课题组名称	LHD高效洁净燃烧(CPCR)
论文分区	一类
引用统计	被引频次：2[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://dspace.imech.ac.cn/handle/311007/71948
专题	高温气体动力学国家重点实验室
通讯作者	Wei, XL (reprint author), Chinese Acad Sci, Inst Mech, State Key Lab High Temp Gas Dynam, Beijing 100190, Peoples R China.
推荐引用方式 GB/T 7714	Wu, Dongyin,Wang, Yuhao,Wei XL,et al. Experimental investigation and numerical simulation of CO oxidation with HCl addition[J]. FUEL,2016,179:221-228.
APA	Wu, Dongyin,Wang, Yuhao,魏小林,李森,Guo, Xiaofeng,&Wei, XL .(2016).Experimental investigation and numerical simulation of CO oxidation with HCl addition.FUEL,179,221-228.
MLA	Wu, Dongyin,et al."Experimental investigation and numerical simulation of CO oxidation with HCl addition".FUEL 179(2016):221-228.

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