Interface Aspects in All-Solid-State Li-Based Batteries Reviewed | |
Chen, Chunguang1; Jiang, Ming1,2; Zhou, Tao3; Raijmakers, Luc1; Vezhlev, Egor4; Wu, Baolin1,5; Schuelli, Tobias U6; Danilov, Dmitri L1,2; Wei YJ(魏宇杰)7,8; Eichel, Ruediger-A1,5; Notten, Peter H L1,2,9 | |
发表期刊 | ADVANCED ENERGY MATERIALS |
2021-02-18 | |
页码 | 55 |
ISSN | 1614-6832 |
摘要 | Extensive efforts have been made to improve the Li-ionic conductivity of solid electrolytes (SE) for developing promising all-solid-state Li-based batteries (ASSB). Recent studies suggest that minimizing the existing interface problems is even more important than maximizing the conductivity of SE. Interfaces are essential in ASSB, and their properties significantly influence the battery performance. Interface problems, arising from both physical and (electro)chemical material properties, can significantly inhibit the transport of electrons and Li-ions in ASSB. Consequently, interface problems may result in interlayer formation, high impedances, immobilization of moveable Li-ions, loss of active host sites available to accommodate Li-ions, and Li-dendrite formation, all causing significant storage capacity losses and ultimately battery failures. The characteristic differences of interfaces between liquid- and solid-type Li-based batteries are presented here. Interface types, interlayer origin, physical and chemical structures, properties, time evolution, complex interrelations between various factors, and promising interfacial tailoring approaches are reviewed. Furthermore, recent advances in the interface-sensitive or depth-resolved analytical tools that can provide mechanistic insights into the interlayer formation and strategies to tailor the interlayer formation, composition, and properties are discussed. |
关键词 | all‐ solid‐ state batteries depth profiling interfaces interfacial resolution lithium detection |
DOI | 10.1002/aenm.202003939 |
收录类别 | SCI ; EI |
语种 | 英语 |
WOS记录号 | WOS:000618968600001 |
WOS研究方向 | Chemistry ; Energy & Fuels ; Materials Science ; Physics |
WOS类目 | Chemistry, Physical ; Energy & Fuels ; Materials Science, Multidisciplinary ; Physics, Applied ; Physics, Condensed Matter |
资助项目 | LImeSI project[DB001702] ; Center for Nanoscale Materials, a U.S. Department of Energy Office of Science User Facility[DE-AC02-06CH11357] ; Projekt DEAL |
项目资助者 | LImeSI project ; Center for Nanoscale Materials, a U.S. Department of Energy Office of Science User Facility ; Projekt DEAL |
论文分区 | 一类 |
力学所作者排名 | 1 |
RpAuthor | Chen, Chunguang ; Wei, YJ |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://dspace.imech.ac.cn/handle/311007/86065 |
专题 | 非线性力学国家重点实验室 |
作者单位 | 1.Forschungszentrum Julich IEK 9, D-52425 Julich, Germany; 2.Eindhoven Univ Technol, POB 513, NL-5600 MB Eindhoven, Netherlands; 3.Argonne Natl Lab, Nanosci & Technol Div, Lemont, IL 60439 USA; 4.Forschungszentrum Julich, Julich Ctr Neutron Sci JCNS 4, D-85748 Garching, Germany; 5.Rhein Westfal TH Aachen, Inst Phys Chem, D-52074 Aachen, Germany; 6.ID01 ESRF, CS 40220, F-38043 Grenoble 9, France; 7.Chinese Acad Sci, Inst Mech, LNM, Beijing 100190, Peoples R China; 8.Univ Chinese Acad Sci, Sch Engn Sci, Beijing 100049, Peoples R China; 9.Univ Technol Sydney, Ctr Clean Energy Technol, Sydney, NSW 2007, Australia |
推荐引用方式 GB/T 7714 | Chen, Chunguang,Jiang, Ming,Zhou, Tao,et al. Interface Aspects in All-Solid-State Li-Based Batteries Reviewed[J]. ADVANCED ENERGY MATERIALS,2021:55. |
APA | Chen, Chunguang.,Jiang, Ming.,Zhou, Tao.,Raijmakers, Luc.,Vezhlev, Egor.,...&Notten, Peter H L.(2021).Interface Aspects in All-Solid-State Li-Based Batteries Reviewed.ADVANCED ENERGY MATERIALS,55. |
MLA | Chen, Chunguang,et al."Interface Aspects in All-Solid-State Li-Based Batteries Reviewed".ADVANCED ENERGY MATERIALS (2021):55. |
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