The effects of particle size on flameless combustion characteristics and NOx emissions of semi-coke with coal | |
Ding, Hongliang1,2; Ouyang, Ziqu1,2; Zhang, Xiaoyu1,3; Zhu SJ(朱书骏)1,4 | |
发表期刊 | FUEL |
2021-08-01 | |
卷号 | 297页码:13 |
ISSN | 0016-2361 |
摘要 | The experiments of the effect of particle size on flameless combustion characteristics and NOx emissions of Shenmu semi-coke were launched on a bench-scale coal preheating combustion test rig. The results revealed that the difference of fuel particle size greatly influenced the yield of each component in high-temperature coal gas and the reactive activity of coal char, thus subsequently affecting the final combustion process and NOx emissions. The specific surface area and pore volume of Shenmu semi-coke were both significantly increased after preheated, leading to a better reactivity and the improved combustion performance, especially when d(50) (the mean particle size) = 163.84 mu m, where the temperature of the down-fired combustor reached the highest. The different particle size of Shenmu semi-coke resulted in different preheating temperature, which further affected the content of each component in the high-temperature coal gas. During the self-preheating process, most volatile matter and fuel bound N were separated out and the released N was mainly converted to N-2 and NH3, besides the conversion rate of each component (C, H, N and V) was the highest when d(50) = 100.17 mu m. Additionally, all experimental conditions achieved flameless combustion, with a transparent combustion area, but no flame front visible to the naked eye, and the highest combustion efficiency was 98.23% when d(50) = 163.84 mu m with the brightest flame image. It was discovered in this experimental that there was a critical value (d(50) = 198.54 mu m) of Shenmu semi-coke particles. When the particle size was lower than or higher than the critical value, NOx generated by combustion would decrease. The lowest NOx emission was 89.46 mg/m3 (@6% O-2) when d(50) was 35.34 mu m. |
关键词 | Particle size Self-preheating Flameless combustion NOx emissions |
DOI | 10.1016/j.fuel.2021.120758 |
收录类别 | SCI ; EI |
语种 | 英语 |
WOS记录号 | WOS:000647587300002 |
关键词[WOS] | CIRCULATING FLUIDIZED-BED ; GASIFICATION FLY-ASH ; DOWN-FIRED BOILER ; PULVERIZED-COAL ; LABORATORY FURNACE ; AIR ; REDUCTION ; OXIDATION ; FLOW |
WOS研究方向 | Energy & Fuels ; Engineering |
WOS类目 | Energy & Fuels ; Engineering, Chemical |
资助项目 | National Key R&D Program of China[2017YFB0602001] ; National Natural Science Foundation of China[52006233] ; Youth Innovation Promotion Association, CAS[2019148] |
项目资助者 | National Key R&D Program of China ; National Natural Science Foundation of China ; Youth Innovation Promotion Association, CAS |
论文分区 | 一类 |
力学所作者排名 | 3+ |
RpAuthor | Ouyang, Ziqu |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://dspace.imech.ac.cn/handle/311007/86721 |
专题 | 高温气体动力学国家重点实验室 |
通讯作者 | Ouyang, Ziqu |
作者单位 | 1.Chinese Acad Sci, Inst Engn Thermophys, 11Beisihuanxi Rd, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Univ Sci & Technol China, Hefei 230026, Peoples R China 4.Chinese Acad Sci, Inst Mech, State Key Lab High Temp Gas Dynam, Beijing 100190, Peoples R China |
推荐引用方式 GB/T 7714 | Ding, Hongliang,Ouyang, Ziqu,Zhang, Xiaoyu,et al. The effects of particle size on flameless combustion characteristics and NOx emissions of semi-coke with coal[J]. FUEL,2021,297:13. |
APA | Ding, Hongliang,Ouyang, Ziqu,Zhang, Xiaoyu,&Zhu SJ.(2021).The effects of particle size on flameless combustion characteristics and NOx emissions of semi-coke with coal.FUEL,297,13. |
MLA | Ding, Hongliang,et al."The effects of particle size on flameless combustion characteristics and NOx emissions of semi-coke with coal".FUEL 297(2021):13. |
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