Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting

doi:10.1021/acsmaterialslett.0c00549

	Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting
	Yuan, Cheng-Zong ; Hui, Kwan San 9; Yin, Hong 1; Zhu, Siqi 2; Zhang, Jintao 3; Wu, Xi-Lin ; Hong, Xiaoting 5; Zhou, Wei 6; Fan, Xi 7; Bin F(宾峰); Chen, Fuming ; Hui, Kwun Nam
发表期刊	ACS MATERIALS LETTERS
	2021-07
卷号	3 期号:6 页码:752-780
摘要	Efficient and low-cost transition-metal (TM)-based electrocatalysts have been of great importance for producing hydrogen (H-2) and oxygen (O-2) via electrocatalytic water (H2O) splitting to ameliorate global energy and environmental problems. However, TM-based materials generally suffer from unsatisfactory electrocatalytic activity because of their relatively low conductivity and unregulated electronic structure. Therefore, the electronic structure engineering of electrocatalysts is an efficient strategic approach to enhance catalytic performances and stabilities. In this review, recent experimental and theoretical advances in the intrinsic electronic structure regulation of TM-based nanomaterials are summarized in terms of preparation methods and underlying natures to boost hydrogen evolution reaction and oxygen evolution reaction. A systematic discussion is conducted on engineering strategies for TM-based nanomaterials to regulate their electronic structures, optimize their adsorption ability of reaction intermediates, and reduce reaction barrier. The existing challenges and perspectives of TM-based electrocatalysts are highlighted to provide new insights into technological advancement for hydrogen production.
学科领域	Materials Science, Multidisciplinary
DOI	10.1021/acsmaterialslett.0c00549
收录类别	SCI
语种	英语
WOS记录号	WOS:000661316200007
项目资助者	Science and Technology Development Fund, Macau SAR [0191/2017/A3, 0041/2019/A1, 0046/2019/AFJ, 0021/2019/AIR] ; University of Macau [MYRG2017-00216-FST, MYRG2018-00192-IAPME] ; UEA ; Zhejiang Province Basic Public Welfare Research Project [LGF19B070006] ; Science and Technology Program of Guangzhou [2019050001] ; National Key Research and Development Program of China ; Scientific and Technological Plan of Guangdong Province [2018A050506078, 2018B050502010] ; Department of Education of Guangdong Province [2019KZDXM014, 2018KTSCX047] ; China Postdoctoral Science Foundation [2019M662955] ; Natural Science Foundation of Guangdong province [2019A1515011615] ; SCNU Outstanding Young Scholar Project [8S0256] ; UM Macao Postdoctoral Fellowship and Associateship ; Pearl River Talent Program [2019QN01L951]
论文分区	一类
力学所作者排名	3+
RpAuthor	Hui, KN (corresponding author), Univ Macau, Inst Appl Phys & Mat Engn, Minist Educ, Joint Key Lab, Taipa 999078, Macau Sar, Peoples R China. ; Hui, KS (corresponding author), Univ East Anglia, Fac Sci, Sch Engn, Norwich NR4 7TJ, Norfolk, England. ; Chen, FM (corresponding author), South China Normal Univ, Sch Phys & Telecommun Engn, State Key Lab Opt Informat Phys & Technol, Guangzhou 510006, Peoples R China.
引用统计	被引频次：62[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://dspace.imech.ac.cn/handle/311007/90232
专题	高温气体动力学国家重点实验室
作者单位	1.Univ Macau, Inst Appl Phys & Mat Engn, Minist Educ, Joint Key Lab, Taipa 999078, Macau Sar, Peoples R China 2.Huazhong Univ Sci & Technol, Appl Mat, Wuhan 430074, Hubei, Peoples R China 3.Anhui Univ Technol, Maanshan, Anhui, Peoples R China 4.Shandong Univ, Sch Chem & Chem Engn, Jinan 250061, Peoples R China 5.Zhejiang Normal Univ, Coll Geog & Environm Sci, Jinhua 321004, Zhejiang, Peoples R China 6.Zhejiang Sci Tech Univ, Dept Chem, Hangzhou 310018, Peoples R China 7.Xiamen Univ, Dept Mech & Elect Engn, Xiamen 361005, Peoples R China 8.Chinese Acad Sci, Ningbo Inst Mat Technol Engn, Ningbo 315201, Peoples R China 9.Chinese Acad Sci, Inst Mech, State Key Lab High Temp Gas Dynam, Beijing 100190, Peoples R China 10.Univ East Anglia, Fac Sci, Sch Engn, Norwich NR4 7TJ, Norfolk, England
推荐引用方式 GB/T 7714	Yuan, Cheng-Zong,Hui, Kwan San,Yin, Hong,et al. Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting[J]. ACS MATERIALS LETTERS,2021,3,6,:752-780.
APA	Yuan, Cheng-Zong.,Hui, Kwan San.,Yin, Hong.,Zhu, Siqi.,Zhang, Jintao.,...&Hui, Kwun Nam.(2021).Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting.ACS MATERIALS LETTERS,3(6),752-780.
MLA	Yuan, Cheng-Zong,et al."Regulating Intrinsic Electronic Structures of Transition-Metal-Based Catalysts and the Potential Applications for Electrocatalytic Water Splitting".ACS MATERIALS LETTERS 3.6(2021):752-780.

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