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硝基甲烷振动能量弛豫的集体模型
Alternative TitleVibrational Energy Relaxation of Nitromethane in Collective Model
赵波; 崔季平; 樊菁
Source Publication计算物理
2010-07-25
Volume27Issue:4Pages:579-585
ISSN1001-246X
Abstract用分子动力学方法结合Dlott等人提出的"门槛模"理论研究集体相互作用下硝基甲烷振动能量弛豫过程.其中振动冷却过程与实验符合的很好.在振动激发过程的分子动力学模拟中观测到与实验一致的基频频移现象.用分子动力学方法从微观上详细地描述出分子"门槛模"振动激发过程.研究表明,在高温高压作用下,集体作用效应对多原子振动激发具有不可忽视的作用,能量传递过程中除了基频的作用外,强烈的非线性相互作用引起的振动模泛频也携带有大量的振动能,这些泛频也对分子振动能量传递产生重要影响.
Keyword振动能量弛豫 硝基甲烷 集体作用 分子动力学
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Indexed ByEI ; CSCD
Language中文
CSCD IDCSCD:3902919
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Document Type期刊论文
Identifierhttp://dspace.imech.ac.cn/handle/311007/43850
Collection高温气体动力学国家重点实验室
Corresponding Author赵波
Recommended Citation
GB/T 7714
赵波,崔季平,樊菁. 硝基甲烷振动能量弛豫的集体模型[J]. 计算物理,2010,27(4):579-585.
APA 赵波,崔季平,&樊菁.(2010).硝基甲烷振动能量弛豫的集体模型.计算物理,27(4),579-585.
MLA 赵波,et al."硝基甲烷振动能量弛豫的集体模型".计算物理 27.4(2010):579-585.
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