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Synthesis and hydrogen-storage performance of interpenetrated MOF-5/MWCNTs hybrid composite with high mesoporosity
Jiang H(姜恒); Feng YF(冯亚菲); Chen M(陈猛); Wang YR(王育人); Wang, YR (reprint author), Chinese Acad Sci, Inst Mech, Key Lab Micrograv Sci, Beijing 100190, Peoples R China.
2013-08-21
发表期刊International Journal of Hydrogen Energy
卷号38期号:25页码:10950-10955
ISSN0360-3199
摘要Metal-organic frameworks (MOFs) exhibiting high surface area and tunable pore size own broad application prospects. Compared with existing MOFs, MOF-5 [Zn4O(bdc)3] is a promising hydrogen storage material due to high H2 uptake capacity and thermostability. However, further wider applications of MOF-5 have been limited because atmospheric moisture levels cause MOF-5 instability. MOF-5 and multi-walled carbon nanotubes (MWCNTs) hybrid composite (denoted MOFMC) can enhance stability toward ambient moisture and improve hydrogen storage capacity. In this paper, the MOFMC, which has an interpenetrated structure with high mesoporosity, was synthesized. The MOFMC is denoted as Int-MOFMC-meso. It stored 2.02 wt% H2 at 77 K under 1 bar, which is higher than the MOF-5 with similar structure and the earlier reported MOFMC material. Moreover, the Int-MOFMC-meso can also show more excellent performance of thermostability and moisture stability than the MOF-5 with similar structure.
关键词Metal-organic Frameworks Interpenetrated Structure Hydrogen-storage Multi-walled Carbon Nanotubes High Mesoporosity
学科领域新型材料的力学问题
DOI10.1016/j.ijhydene.2013.03.044
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收录类别SCI ; EI
语种英语
WOS记录号WOS:000324563100096
关键词[WOS]METAL-ORGANIC FRAMEWORKS ; NANOPOROUS MATERIALS ; SORPTION PROPERTIES ; ADSORPTION ; CARBON ; MOF-5 ; INCLUSION ; BEHAVIORS ; DESIGN ; SIZE
WOS研究方向Chemistry ; Electrochemistry ; Energy & Fuels
WOS类目Chemistry, Physical ; Electrochemistry ; Energy & Fuels
项目资助者The authors wish to acknowledge the support from the National Natural Science Foundation of China (Nos. 11202211 and 11272315).
课题组名称中科院国家微重力实验室
引用统计
被引频次:18[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://dspace.imech.ac.cn/handle/311007/47434
专题国家微重力实验室
通讯作者Wang, YR (reprint author), Chinese Acad Sci, Inst Mech, Key Lab Micrograv Sci, Beijing 100190, Peoples R China.
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GB/T 7714
Jiang H,Feng YF,Chen M,et al. Synthesis and hydrogen-storage performance of interpenetrated MOF-5/MWCNTs hybrid composite with high mesoporosity[J]. International Journal of Hydrogen Energy,2013,38(25):10950-10955.
APA 姜恒,冯亚菲,陈猛,王育人,&Wang, YR .(2013).Synthesis and hydrogen-storage performance of interpenetrated MOF-5/MWCNTs hybrid composite with high mesoporosity.International Journal of Hydrogen Energy,38(25),10950-10955.
MLA 姜恒,et al."Synthesis and hydrogen-storage performance of interpenetrated MOF-5/MWCNTs hybrid composite with high mesoporosity".International Journal of Hydrogen Energy 38.25(2013):10950-10955.
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