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Title:
Synthesis and hydrogen-storage performance of interpenetrated MOF-5/MWCNTs hybrid composite with high mesoporosity
Author: Jiang H(姜恒); Feng YF(冯亚菲); Chen M(陈猛); Wang YR(王育人)
Source: International Journal of Hydrogen Energy
Issued Date: 2013-08-21
Volume: 38, Issue:25, Pages:10950-10955
Abstract: Metal-organic frameworks (MOFs) exhibiting high surface area and tunable pore size own broad application prospects. Compared with existing MOFs, MOF-5 [Zn4O(bdc)3] is a promising hydrogen storage material due to high H2 uptake capacity and thermostability. However, further wider applications of MOF-5 have been limited because atmospheric moisture levels cause MOF-5 instability. MOF-5 and multi-walled carbon nanotubes (MWCNTs) hybrid composite (denoted MOFMC) can enhance stability toward ambient moisture and improve hydrogen storage capacity. In this paper, the MOFMC, which has an interpenetrated structure with high mesoporosity, was synthesized. The MOFMC is denoted as Int-MOFMC-meso. It stored 2.02 wt% H2 at 77 K under 1 bar, which is higher than the MOF-5 with similar structure and the earlier reported MOFMC material. Moreover, the Int-MOFMC-meso can also show more excellent performance of thermostability and moisture stability than the MOF-5 with similar structure.
Keyword: Metal-organic frameworks ; Interpenetrated structure ; Hydrogen-storage ; Multi-walled carbon nanotubes ; High mesoporosity
Language: 英语
Indexed Type: SCI ; EI
Corresponding Author: Wang, YR (reprint author), Chinese Acad Sci, Inst Mech, Key Lab Micrograv Sci, Beijing 100190, Peoples R China.
Correspondent Email: yurenwang@imech.ac.cn
DOI: 10.1016/j.ijhydene.2013.03.044
Related URLs: 查看原文
DOC Type: Article; Proceedings Paper
WOS Subject: Chemistry, Physical ; Electrochemistry ; Energy & Fuels
WOS Subject Extended: Chemistry ; Electrochemistry ; Energy & Fuels
WOS Keyword Plus: METAL-ORGANIC FRAMEWORKS ; NANOPOROUS MATERIALS ; SORPTION PROPERTIES ; ADSORPTION ; CARBON ; MOF-5 ; INCLUSION ; BEHAVIORS ; DESIGN ; SIZE
WOS ID: WOS:000324563100096
ISSN: 0360-3199
Rank: [Jiang, Heng; Feng, Yafei; Chen, Meng; Wang, Yuren] Key Laboratory of Microgravity, Institute of Mechanics, Chinese Academy of Sciences, No.15 Beisihuanxi Road, Beijing 100190, PR China
Subject: 固体力学::新型材料的力学问题
Department: 中科院国家微重力实验室
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Content Type: 期刊论文
URI: http://dspace.imech.ac.cn/handle/311007/47434
Appears in Collections:国家微重力实验室_期刊论文

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Recommended Citation:
Jiang H,Feng YF,Chen M,et al. Synthesis and hydrogen-storage performance of interpenetrated MOF-5/MWCNTs hybrid composite with high mesoporosity[J]. International Journal of Hydrogen Energy,2013-08-21,38(25):10950-10955.
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